Suggestions by @jasonadams1

Victor Buono

as King Tut in Batman (1970)

Eli Wallach

as Mr. Freeze in Batman (1970)

Anthony Perkins

as Scarecrow in Batman (1970)

Dean Martin

as Joe Chill in Batman (1970)

Frank Sinatra

as Lew Moxon in Batman (1970)

Vincent Price

as Egghead in Batman (1970)

Clint Eastwood

as Two-Face in Batman (1970)

Ann-Margret

as Poison Ivy in Batman (1970)

Julie Newmar

as Catwoman in Batman (1970)

Frank Gorshin

as The Riddler in Batman (1970)

Burgess Meredith

as The Penguin in Batman (1970)

Andy Griffith

as Commissioner Murphy in Batman (1970)

Cesar Romero

as The Joker in Batman (1970)

Stafford Repp

as Chief O'Hara in Batman (1970)

Neil Hamilton

as Mayor Gordon in Batman (1970)

Alan Napier

as Alfred Pennyworth in Batman (1970)

Yvonne Craig

as Batgirl in Batman (1970)

Burt Ward

as Robin in Batman (1970)

Adam West

as Batman in Batman (1970)

Alan Napier

as Alfred Pennyworth in Batman 2 (1970)